Wow. That pull looks as bad as some of the pep helmets I've seen.
Now, I have no molding experience, but:
- Could you please post some pictures of the mold, and everything related to the mold,
- Did you make sure that the Rebound mold was snug against the inside of the jacket?
- When you removed it, was is that way, or did is smush after you pulled it out?
- Did you make sure to keep rotating the mold until it was hard enough to keep it's shape?
- Did you use the right plastic to catalyst ratio?
My guess is that you didn't rotate the model enough, and set it down right-side-up, and the top smushed down inside the mold because it was still soft enough to smush.