well, from what i understand (not having gotten to that stage yet in my armour build), you can take some primer (i hear grey works best) and spray paint the outside of the helmet, apparently the primer helps to bring out the imperfections that need attention, then from there you sand down the problem areas and apply the necessary amount of bondo to bring the helmet as close to what it looks like in the game as possible. (example, for making a smooth curve out of the edgy curve that pepakura pieces make)
hope that helped =D, and good luck on the rest of your build